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1.
J Environ Manage ; 329: 117058, 2023 Mar 01.
Artigo em Inglês | MEDLINE | ID: mdl-36528944

RESUMO

Aquatic sediment polluted by potentially toxic elements (PTEs) from mining activities represents a potential health "time bomb" for humans and the local ecology, but the integrated analysis of pollution and hazards of PTEs in sediment around typical metal mines in China is limited. Presently, the associated pollution status, spatial distribution, and ecological and health hazards of Cd, Cu, Zn, Pb, Cr, and As were investigated through index evaluation, spatial analysis, health risk assessment models, and Monte Carlo simulation. Overall, the sediment exhibited varying degrees of PTE contamination; notably, the level of Cd was 104.85 times higher than its background value, and it became the most enriched element in the surveyed sediment, followed in descending order by Cu, As, Zn, Pb, and Cr. Nationally, over 64.5% of metal-mining-affected sediment presented a very high ecological risk, contributed mostly by Cd (43.2%-98.7%) followed by As, Pb, and Cu; the risk contributed by both Cr and Zn was found to be negligible. The adverse health risk posed to children by most sediment was 1.72 and 6.46 times higher than that posed to adults for cancerous and noncancerous risks, respectively. The potential noncarcinogenic risks were mainly caused by As, which contributed over 78.9% of the Hazard Index values, then followed by Pb (>9.3%). For both children and adults, the carcinogenic risk of PTEs decreased in the following order: As > Cd > Cr > Pb. The investigated sediment was found seriously affected by nearby metal mines, especially those in regions with long-term and large-scale nonferrous-metal-mining activities. This study could provide a reference for policymakers to develop control strategies for PTE pollution in sediment around mining areas.


Assuntos
Metais Pesados , Poluentes do Solo , Criança , Adulto , Humanos , Metais Pesados/análise , Monitoramento Ambiental , Cádmio , Chumbo , Solo , Poluentes do Solo/análise , China , Medição de Risco
2.
Artigo em Inglês | MEDLINE | ID: mdl-36231503

RESUMO

To better protect lacustrine ecologies and understand the evolutionary process of lake environments, it is critical to study the interacting mechanisms between lakes and the surrounding groundwater. The Wuliangsu Lake watershed is the largest wetland in the Yellow River basin and is the discharge area of the Hetao Irrigation District (HID), which is one of the three largest agricultural production areas in China. Due to the influence of human activities, the discharge water from the HID has led to the deterioration of the Wuliangsu Lake ecology and the degradation of the lake environment. Based on long-term observation data and water sampling data collected in 2021, a water-salt equilibrium model was used to analyze the recharge rate of groundwater to the lake. The contribution rate of groundwater to lake recharge in the study area was calculated with a Bayesian mixing model by combining D and 18O stable isotope data. Furthermore, the environmental evolutionary process of the lake was also analyzed using the collected water quality data. The results show that channel drainage was the main source of recharge to Wuliangsu Lake, accounting for more than 75%, while groundwater contributed less than 5% of lake recharge. After implementing the ecological water supplement plan, the concentration of various ions in the lake decreased, the concentration of the total dissolved solids (TDS) in the lake decreased from 1.7 g/L in 2016 to 1.28 g/L in 2021, and the ecological environment was improved. The contribution of groundwater to lake recharge was quantitatively analyzed. The results of this study can facilitate the development of vital strategies for preventing the further deterioration of lake water quality and for protecting wetland ecologies.


Assuntos
Água Subterrânea , Poluentes Químicos da Água , Teorema de Bayes , China , Monitoramento Ambiental/métodos , Água Subterrânea/análise , Humanos , Isótopos/análise , Lagos , Rios , Cloreto de Sódio/análise , Poluentes Químicos da Água/análise
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